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That should sort by the title in the ID3 tag. If your filenames are in the format of Artist - Title, then you want to sort by filename. That is what I do.
I have several folders in Finder, but I can find no way of keeping them in alphabetical order. They move according to when they were last accessed, which, for my work, is confusing.
If you download a lot of documents, pictures, music, and photos every day, you will end up having a lot of files in your Downloads folders and you may have to manually move or sort these files to ...
The three sorting tools do have three distinct functions: Arrange By lets you organize files into groups. The Sort By option lets you choose how your files are sorted (by name, date, etc.).